Publications

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• Magnetic, electronic, and structural investigation of the strongly correlated Y$_{1-x}$Sm$_{x}$Co$_5$ system

  F. Passos, D. Cornejo, G. J. Nilsen, V. Martelli, J. Larrea Jiménez

  SciPost Phys. Proc. 11, 021 (2023) · published 6 June 2023 | Toggle abstract · pdf

  SmCo$_5$ and YCo$_5$ are isostructural compounds both showing large magnetocrystalline anisotropy, where the former originates mainly from the crystal-electric field and magnetic interactions. We investigate the contribution of both interactions by partially substituting Y by Sm in as-cast polycrystalline Y$_{1-x}$Sm$_{x}$Co$_5$ (with $x$=0.00, 0.12, 0.18, 0.31, and 0.40) and measuring their structural, magnetic, and electrical properties through X-ray diffraction, magnetization, and electrical transport measurements. Our results suggest an interplay between microstructure strain in as-cast samples and the electronic and magnetic interactions.

• Composition dependence of the specific heat of FeSi

  Carolina Burger, Andreas Bauer, Christian Pfleiderer

  SciPost Phys. Proc. 11, 020 (2023) · published 6 June 2023 | Toggle abstract · pdf

  Recently, a high-mobility surface conduction channel and in-gap states were identified in the correlated small-gap semiconductor FeSi using electrical transport measurements and high-resolution tunneling spectroscopy. The mobility of the charge carriers in the surface channel is quantitatively reminiscent of topological insulators, but displays a lack of sensitivity to the presence of ferromagnetic impurities as studied by means of a series of single crystals with slightly different starting compositions. Here, we report measurements of the specific heat of these crystals. At low temperatures, a shallow maximum is observed in the specific heat divided by temperature. This maximum is suppressed under magnetic field, characteristic of a Schottky anomaly associated with magnetic impurities. In comparison, the height of this maximum decreases with increasing initial iron content.

• In-plane Fermi surface mapping of ZrSiS and HfSiS by de Haas-van Alphen oscillations

  Bruno Gudac, Mihovil Bosnar, Filip Orbanić, Trpimir Ivšić, Ivan Kokanović, Mario Novak

  SciPost Phys. Proc. 11, 019 (2023) · published 6 June 2023 | Toggle abstract · pdf

  We have conducted a comprehensive experimental investigation of the in-plane de Haas van Alphen quantum oscillations in ZrSiS and HfSiS and compared the results to the ab-initio calculations. We found a moderately good agreement for a set of frequencies located between 100 T and 200 T. These could be associated with extremal orbitals of the electron pockets located around the $k_z=\pm\pi/2c$ planes at the edge of the 1st Brillouin zone. In contrast, the experimentally detected low-frequency set of oscillations found around 20 T could not be reproduced by the calculations. Further refinement of the ab-initio calculation has to be conducted to fully capture all the observed features of the Fermi surface in ZrSiS and HfSiS.

• Pressure-dependent structural and electronic instabilities in LaSb$_2$

  Theodore I. Weinberger, Christian K. de Podesta, Jiasheng Chen, Stephen A. Hodgson, F. Malte Grosche

  SciPost Phys. Proc. 11, 018 (2023) · published 6 June 2023 | Toggle abstract · pdf

  LaSb$_2$ exhibits a large, non-saturating, linear magnetoresistance at low temperatures, defying the expectations of Fermi liquid theory. This is thought to be caused by charge density wave order emerging below an abrupt, hysteretic anomaly in the resistivity at $\sim$ 355 K. We find that, under hydrostatic pressure, this anomaly becomes much more pronounced, develops strong hysteresis, and shifts rapidly towards lower temperatures. The anomaly is fully suppressed by only 6 kbar. Moreover, we observe a second transition anomaly at lower temperature, which likewise disappears under pressure. These findings are discussed in the context of a structural transition recently discovered in the sister material CeSb$_2$ and of density functional theory calculations, which indicate that the SmSb$_2$-type structure adopted by LaSb$_2$ at ambient conditions is unstable at moderate applied pressures.

• Local investigation of the crystal electric field ground-state in CeCu(Sb,Bi)$_2$ heavy fermions

  Davi Zau, G. S. Freitas, P. G. Pagliuso, R. R. Urbano

  SciPost Phys. Proc. 11, 017 (2023) · published 6 June 2023 | Toggle abstract · pdf

  In this work, we performed systematic Nuclear Magnetic Resonance (NMR) and magnetic susceptibility experiments in CeCuSb$_2$ single-crystals. The main findings were compared to previous report for CeCuBi$_2$. The NMR spectra and transferred hyperfine coupling for the $^{63}$Cu nuclei were obtained aiming to observe their correlation with the crystal electric field (CEF) effects on the Ce$^{3+}$ ($J=5/2$) multiplet. Besides, in an attempt to elucidate the magnetic structure through NMR measurements at different magnetic fields orientations, we observed a magnetic transition at $T\approx 8\,$K higher than the Néel temperature $T_N$ measured by magnetic susceptibility indicating the development of short-range magnetic ordering above T$_N$. In addition, the wipe out of the main NMR resonance line and a persistent spin-echo signal throughout the whole frequency-swept range suggest the possibility of an incommensurate magnetic structure in CeCuSb$_2$. Furthermore, the small transferred hyperfine coupling constant found for CeCuSb$_2$ indicates a scenario with more localized Ce$^{3+}$ 4f electrons than for CeMIn$_5$ (M $=$ Co,Rh,Ir) heavy fermions family. Additionally, subtle changes in the hybridization between the $^{63}$Cu with the 4f$^1$ Ce$^{3+}$ electrons in distinct magnetic field orientations allowed us to provide detailed information and map out the 4f CEF orbital ground-state of CeCu(Sb,Bi)$_2$ via NMR measurements.

• EPR and SQUID interrogations of Cr(III) trimer complexes in the MIL-101(Cr) and bimetallic MIL-100(Al/Cr) MOFs

  Kavipriya Thangavel, Andrea Folli, Michael Ziese, Steffen Hausdorf, Stefan Kaskel, Damien M. Murphy, Andreas Pöppl

  SciPost Phys. Proc. 11, 016 (2023) · published 6 June 2023 | Toggle abstract · pdf

  Herein, electron paramagnetic resonance (EPR) spectroscopy at X- (9.4 GHz), Q- (34 GHz) and W-band (95 GHz), and superconducting quantum interference device (SQUID) measurements on antiferromagnetically coupled metal trimers in MIL-101(Cr) and MIL-100(Al$_{0.8}$Cr$_{0.2}$) MOFs were investigated. At low temperatures, the Cr(III) trimers exhibit a Dzyaloshinsky-Moriya (D-M) interaction, and have a total spin state S$_T = 1/2$.

• Field-induced local Fermi-liquid states in the underscreened Kondo model for Eu compounds

  Shingo Kuniyoshi, Ryousuke Shiina

  SciPost Phys. Proc. 11, 015 (2023) · published 6 June 2023 | Toggle abstract · pdf

  We have studied an underscreened Kondo model for the impurity spin $S=7/2$ capturing the $4f$ characteristics of a nearly divalent Eu ion. By using the numerical renormalization group method, it is shown that an unusual heavy-fermion state is induced from the underscreened spin state when a weak crystal field is introduced. It is also found that the application of the magnetic field enhances the effective mass of the heavy fermions, reflecting the field-induced level crossing of the spin states. We will discuss the mechanism of these mass enhancements in terms of a realization of the two-stage Kondo effect.

• Josephson effects between the Kitaev ladder superconductors

  Osamu Kanehira, Hiroki Tsuchiura

  SciPost Phys. Proc. 11, 014 (2023) · published 6 June 2023 | Toggle abstract · pdf

  The two-leg ladder system consisting of the Kitaev chains is known to exhibit a richer phase diagram than that of the single chain. We theoretically investigate the variety of the Josephson effects between the ladder systems. We consider the Josephson phase difference $\theta$ between these two ladder systems as well as the phase difference $\phi$ between the parallel chains in each ladder system. The total energy of the junction at $T = 0$ is calculated by a numerical diagonalization method as functions of $\theta$, $\phi$, and also a transverse hopping $t_{\perp}$ in the ladders. We find that, by controlling $t_{\perp}$ and $\phi$, the junction exhibits not only the fractional Josephson effect for the phase difference $\theta$, but also the usual 0-junction and even $\pi$-junction properties.

• Magnetic properties of a multicomponent intermetallic compound Tb$_{0.25}$Dy$_{0.25}$Ho$_{0.25}$Er$_{0.25}$Al$_2$

  P. K. Jesla, Jeyaramane Arout Chelvane, R. Nirmala

  SciPost Phys. Proc. 11, 013 (2023) · published 6 June 2023 | Toggle abstract · pdf

  Polycrystalline multicomponent Laves phase rare earth intermetallic compound Tb$_{0.25}$ Dy$_{0.25}$Ho$_{0.25}$Er$_{0.25}$Al$_{2}$ has been synthesized by arc-melting and characterized by powder X-ray diffraction, magnetization and heat capacity measurements. The sample has MgCu$_2$-type cubic structure (space group Fd-3m) at 300 K. The compound Tb$_{0.25}$Dy$_{0.25}$Ho$_{0.25}$Er$_{0.25}$ Al$_{2}$ orders ferromagnetically at 50 K (T$_C$). This value is almost equal to the average of the ferromagnetic ordering temperatures of the individual RAl$_2$ (R = Tb, Dy, Ho and Er) compounds. Field dependence of magnetization below T$_C$ indicates soft-ferromagnetic nature. From the magnetization vs field data obtained near T$_C$ and the temperature dependence of heat capacity, low field magnetocaloric effect has been estimated.

  1 citation

• Polarons and bipolarons in a two-dimensional square lattice

  Shanshan Ding, G. A. Domínguez-Castro, Aleksi Julku, Arturo Camacho-Guardian, Georg M. Bruun

  SciPost Phys. 14, 143 (2023) · published 5 June 2023 | Toggle abstract · pdf

  Quasiparticles and their interactions are a key part of our understanding of quantum many-body systems. Quantum simulation experiments with cold atoms have in recent years advanced our understanding of isolated quasiparticles, but so far they have provided limited information regarding their interactions and possible bound states. Here, we show how exploring mobile impurities immersed in a Bose-Einstein condensate (BEC) in a two-dimensional lattice can address this problem. First, the spectral properties of individual impurities are examined, and in addition to the attractive and repulsive polarons known from continuum gases, we identify a new kind of quasiparticle stable for repulsive boson-impurity interactions. The spatial properties of polarons are calculated showing that there is an increased density of bosons at the site of the impurity both for repulsive and attractive interactions. We then derive an effective Schrödinger equation describing two polarons interacting via the exchange of density oscillations in the BEC, which takes into account strong impurity-boson two-body correlations. Using this, we show that the attractive nature of the effective interaction between two polarons combined with the two-dimensionality of the lattice leads to the formation of bound states - i.e. bipolarons. The wave functions of the bipolarons are examined showing that the ground state is symmetric under particle exchange and therefore relevant for bosonic impurities, whereas the first excited state is doubly degenerate and odd under particle exchange making it relevant for fermionic impurities. Our results show that quantum gas microscopy in optical lattices is a promising platform to explore the spatial properties of polarons as well as to finally observe the elusive bipolarons.

  4 citations