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Critical energy landscape of linear soft spheres
by Silvio Franz, Antonio Sclocchi, Pierfrancesco Urbani
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Submission summary
Authors (as registered SciPost users): | Silvio Franz · Antonio Sclocchi |
Submission information | |
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Preprint Link: | https://arxiv.org/abs/2002.04987v2 (pdf) |
Date submitted: | 2020-04-16 02:00 |
Submitted by: | Sclocchi, Antonio |
Submitted to: | SciPost Physics |
Ontological classification | |
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Academic field: | Physics |
Specialties: |
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Approaches: | Theoretical, Computational |
Abstract
We show that soft spheres interacting with a linear ramp potential when overcompressed beyond the jamming point fall in an amorphous solid phase which is critical, mechanically marginally stable and share many features with the jamming point itself. In the whole phase, the relevant local minima of the potential energy landscape display an isostatic contact network of perfectly touching spheres whose statistics is controlled by an infinite lengthscale. Excitations around such energy minima are non-linear, system spanning, and characterized by a set of non-trivial critical exponents. We perform numerical simulations to measure their values and show that, while they coincide, within numerical precision, with the critical exponents appearing at jamming, the nature of the corresponding excitations is richer. Therefore, linear soft spheres appear as a novel class of finite dimensional systems that self-organize into new, critical, marginally stable, states.
Current status:
Reports on this Submission
Report #2 by Anonymous (Referee 1) on 2020-6-2 (Invited Report)
- Cite as: Anonymous, Report on arXiv:2002.04987v2, delivered 2020-06-02, doi: 10.21468/SciPost.Report.1733
Strengths
The manuscript succeeds in arguing, based on simulations of static local minimas in the potential energy landscape, that a granular system with a linear repulsive overlap potential between otherwise non-interacting particles have a critical behavior in 2 (and 3) dimensions, very much like in the infinite-dimensional (mean-field) limit. Furthermore, the potential is such that identical critical behavior is achieved for every density above the jamming transition, due to the strange property of the potential that bringing particles closer together does no further increase the force. Particles either don't or do overlap, it doesn't matter how much! Thus, for all pressures, there is always just enough contact (ie, particles sitting at the boundary from 0-to-1 force) for isostaticity, the pressure just balanced by having more or less particles overlapping. Then, the "gap" on both sides, ie, particles just about to touch, or just barely overlapping, satisfies quite symmetric scaling properties. These are found numerically to be identical to the mean field model. These results are quite convincing. And the concern an area of great interest: jamming in soft matter, which seems to have a very low upper critical dimension and thus might be a great link between glassy mean field theory and actual materials.
Weaknesses
Much of the technical detail (ie, the mean-field underpinnings) is deferred to the references, so a bit of knowledge is required to understand the significance of this work. However, focusing on the numerical results and their physical interpretation (and on 2d, leaving 3d for the appendix) is the right decision, as it makes the manuscript very readable.
Report
I think that this is a very well-conceived project, and I believe it should be published in its current form.
Report #3 by Anonymous (Referee 2) on 2020-5-28 (Invited Report)
- Cite as: Anonymous, Report on arXiv:2002.04987v2, delivered 2020-05-28, doi: 10.21468/SciPost.Report.1739
Report
The authors study a system of soft spheres, in 2 and 3 dimensions, at and beyond the jamming point. Beyond jamming, pairs of spheres interact through a linear ramp potential, which depends on the degree of overlap (negative gap) of the pair of spheres. The linear potential, being singular at zero gap, introduces a series of peculiar properties on the overcompressed amorphous state beyond the jamming point. It is found that local minima of the landscape are isostatic, marginally stable. Then, it is possible to characterize the overcompressed phase from the properties of local
minima of the landscape. After regularizing the singularity of the potential and proceeding to numerical minimizations, the authors show a series of interesting properties of these kind of systems: the whole jammed phase is critical, i.e. beyond the critical packing volume the system self-organizes in a critical state. The distribution of local contact forces and the gap distribution show power law behaviour, with exponents compatible with those at the jamming point. While it is not known if such peculiar behaviour can be seen in realistic systems, the presence of a whole critical phase is interesting in itself. The authors also analyze the nature of non-linear excitations, finding interesting pseudogap behaviour at the extremes of the contact force spectrum.
I found the work interesting, it is well written and describes novel behaviour related to the jamming phenomenology. I have some minor questions, mainly of informative character to the reader, that I suggest the authors to consider including in a final version:
1- How is the jamming transition identified from the properties of locally stable states of the landscape. I mean, what is the change in the stability of these states on approaching the jamming transition ?
2- In page 2, second item, it is said "the spatial fluctuations of the local connectivity of the contact network are hyperuniform''. Although references to previous literature are given, I would find useful to define what "hyperuniform'' means in this context.
3- At the end of Section II, subsection B the authors say "We conclude by noting that while increasing the packing fraction, the fraction of overlaps display a plateau around $\phi \sim 1.5$''. I would say that, if a plateau exists at all in the curve shown if Figure 2, it covers a range between $1.1$ and $1.5$. Do the authors have additional data from say, larger system sizes, to substantiate their claim ?
4- The structure factors of contacts and overlaps are shown in Figure 5. Besides the supression of the structure factor of contacts at large distances, what is the overall interpretation of the behaviour of these quantities. For the same case, why is it constant above a fixed value of the wave vector and what does it mean conceptually ?
5- Finally, the fact that the values of all the critical exponents found are near the mean field ones, both for $d=2$ and $d=3$, implies that mean field universality is generic for finite dimensional jamming systems. Beyond formal statements on the upper critical dimension, what is the physical meaning of this statement in the context of jamming systems ? What is special about criticality in them ?
Report #1 by Anonymous (Referee 3) on 2020-5-4 (Invited Report)
- Cite as: Anonymous, Report on arXiv:2002.04987v2, delivered 2020-05-04, doi: 10.21468/SciPost.Report.1660
Report
Guided by previous mean-field results, the authors study jamming in soft 2D and 3D particle packings where the interparticle potential is a linear ramp. Their main finding is that these systems are critical in a whole interval of packing fractions. This is a very relevant result since, for example, it suggests that mean-field theory (MFT) could be quantitatively accurate also in low dimensions on more than a null-measure region. More implications are clearly described by the authors in the conclusions.
The results are supported via a number of numerical observations on the behavior of these packings. Among those, the fact that they are isostatic and hyperuniform even in the jammed phase. In overcompressed packings, this is possible due to the distinction between kissing and overlapping particles. The indication that correlation lengths are diverging in a whole region of overcompressed packing fractions is evidence for criticality, and provides strong connections to MFT. These connections are explored through the power law scalings of forces and gaps, which are consistent with those found in the related mean-field model (the linear perceptron). Also the density of states is compatible with a finite density of zero modes in the thermodynamics limit, for many packing fractions.
The numerical simulations are performed on smaller systems than in equivalent studies on Harmonic or Hertzian packings, but this may be attributed to the epsilon smoothing that is imposed to the Hamiltonian, which requires to perform several rounds of minimization in order to send epsilon to zero. This does not influence the principal claims of the paper, since an accurate quantitative analysis of scalings is left to future work (it would however be nice to see figure 2 in a log scale, to get an intuition on e.g. the power law $p\sim(\phi-\phi_c)^\beta$ ). The results are given mainly in 2D, with less extensive simulations in 3D that are in reasonable agreement. I could not find where the authors report on how many samples were used to obtain their data (this should be reported).
The manuscript is written in a clear and modular manner, that allows for quick consultation of every single finding. In some cases the figure captions do not contain information such as the system size (amend). In figure 4-left, one of the solid curves is almost completely hidden under the points, and the colors of the solid curves are very similar. I suggest putting the lines on top of the data, using different colors, and using dashes.
The authors succeed in providing physical intuition on their results, and spend time relating them with different kinds of approaches used in the literature.
In summary, the results presented in the article are relevant, well supported by evidence, and well presented. I therefore endorse publication in Scipost Physics.
Requested changes
1- Add numerical details
2- Some captions have missing information on the depicted data
3- It would be nice to see figure 2 in a log scale, to get an intuition on e.g. the power law $p\sim(\phi-\phi_c)^\beta$
4- Improve readability of figure 4