Laser excitation of the 1s-hyperfine transition in muonic hydrogen
by P. Amaro, A. Adamczak, M. Abdou Ahmed, L. Affolter, F. D. Amaro, P. Carvalho, T. -L. Chen, L. M. P. Fernandes, M. Ferro, D. Goeldi, T. Graf, M. Guerra, T. W. Hänsch, C. A. O. Henriques, Y. -C. Huang, P. Indelicato, O. Kara, K. Kirch, A. Knecht, F. Kottmann, Y. -W. Liu, J. Machado, M. Marszalek, R. D. P. Mano, C. M. B. Monteiro, F. Nez, J. Nuber, A. Ouf, N. Paul, R. Pohl, E. Rapisarda, J. M. F. dos Santos, J. P. Santos, P. A. O. C. Silva, L. Sinkunaite, J. -T. Shy, K. Schuhmann, S. Rajamohanan, A. Soter, L. Sustelo, D. Taqqu, L. -B. Wang, F. Wauters, P. Yzombard, M. Zeyen, A. Antognini
Atomic, Molecular and Optical Physics - Experiment
Atomic, Molecular and Optical Physics - Theory
Approaches:
Theoretical, Experimental
Abstract
The CREMA collaboration is pursuing a measurement of the ground-state hyperfine splitting (HFS) in muonic hydrogen ($\mu$p) with 1 ppm accuracy by means of pulsed laser spectroscopy to determine the two-photon-exchange contribution with $2\times10^{-4}$ relative accuracy. In the proposed experiment, the $\mu$p atom which undergoes a laser excitation from the singlet hyperfine state to the triplet hyperfine state, is quenched back to the singlet state by an inelastic collision with a H$_2$ molecule. The resulting increase of kinetic energy after the collisional deexcitation is used as a signature of a successful laser transition between hyperfine states. In this paper we calculate the combined probability that a $\mu$p atom initially in the singlet hyperfine state undergoes a laser excitation to the triplet state followed by a collisional-induced deexcitation back to the singlet state. This combined probability has been computed using the optical Bloch equations including the inelastic and elastic collisions. Omitting the decoherence effects caused by collisions would overestimate the transition probability by more than a factor of three. In this paper, we also account for Doppler effects and the laser bandwidth, and provide the matrix element, the saturation fluence, the elastic and inelastic collision rates for the singlet and triplet states, and the resonance linewidth at the conditions relevant for the hyperfine splitting experiment of the CREMA collaboration. This calculation thus quantifies one of the key unknowns of the HFS experiment, leading to a precise definition of the requirements for the laser system and to an optimization of the hydrogen gas target where $\mu$p is formed and the laser spectroscopy will occur.
