Publications

Order by: publication date number of citations

• Investigation of role of antisite disorder in pristine cage compound FeGa$_3$

  C. Kaufmann Ribeiro , L. Mello , V. Martelli , D. Cornejo, M. B. Silva Neto , E. Fogh , H. M. Rønnow, J. Larrea Jiménez

  SciPost Phys. Proc. 11, 023 (2023) · published 5 September 2023 | Toggle abstract · pdf

  The role of controlled Fe antisite disorder in the narrow gap semiconductor FeGa$_3$ has been investigated. Polycrystalline samples were synthesized by the combination of arc-melting furnace and successive annealing processes. Deviations from occupation numbers of Fe and Ga sites expected in the pristine compound were obtained from X-ray data using Rietveld refinement analysis. Besides that, electrical transport and magnetization measurements reveal that hierarchy in Fe and Ga site disorder tunes the ground state of FeGa$_3$ from paramagnetic semiconductor to a magnetic metal. These findings are discussed inside the framework of Anderson localization in the vicinity of metal-semiconductor transitions and spin fluctuations.

  1 citation

• Structural and magnetic anisotropy in YBa$_2$Cu$_3$O$_7$/La$_{0.67}$Sr$_{0.33}$MnO$_3$ bilayer on SrTiO$_3$ substrate

  Ankita Singh, Ram Prakash Pandeya, Sawani Dutta, Srinivas C. Kandukuri, Kalobaran Maiti

  SciPost Phys. Proc. 11, 007 (2023) · published 5 June 2023 | Toggle abstract · pdf

  We study the magnetic properties and emergence of superconductivity in YBa$_2$Cu$_3$O$_7$ (YBCO)/ La$_{0.67}$Sr$_{0.33}$MnO$_3$ (LSMO) heterostructures. Bilayer films of superconducting layer, YBCO, and ferromagnetic layer, LSMO were grown on SrTiO$_{3}$ (STO) (001) substrate using ultrahigh vacuum Pulsed Laser Deposition system. Magnetization data at 100 K as a function of applied magnetic field shows ferromagnetic behaviour due to the LSMO layer. Cooling below 100 K leads to superconductivity in this material; the onset of superconductivity occurs at a temperature, $T_{c,SC},$ of 86 K for $H_{ext}\perp c$ (in-plane) \& 84 K for $H_{ext}||c$ (out-of-plane) under 100 Oe applied field. In-plane magnetic measurements show significant suppression of diamagnetic behaviour as compared to the out-of-plane measurements. The susceptibility signals are higher for out-of-plane direction. Such strong anisotropy in magnetism and the transition temperatures reveal complex interplay of magnetism and superconductivity in this system and calls for further study in this direction.

  1 citation

• Transport and magnetic properties in the Nd diluted system Y$_{1-x}$Nd$_{x}$Co$_{2}$Zn$_{20}$

  Rikako Yamamoto, Yasuyuki Shimura, Kazunori Umeo, Toshiro Takabatake, Takahiro Onimaru

  SciPost Phys. Proc. 11, 010 (2023) · published 5 June 2023 | Toggle abstract · pdf

  We report the electrical resistivity, specific heat, and magnetization measurements of Y$_{1-x}$Nd$_{x}$Co$_{2}$Zn$_{20}$ for $0.017 \leq x \leq 0.95$. The Schottky-type specific heat peak at around 13 K for all the samples is reproduced by the crystalline electric field model with the $\Gamma_{6}$ doublet ground state of a Nd$^{3+}$ ion. The magnetization and magnetic susceptibility data of the samples for $x \leq 0.06$ are well reproduced by the calculation without intersite magnetic interactions among Nd moments. Therefore, the dilute Nd system Y$_{1-x}$Nd$_{x}$Co$_{2}$Zn$_{20}$ for $x \leq 0.06$ is a good candidate to study on-site interaction of the $\Gamma_{6}$ doublet ground state of 4$f$ electrons with conduction electrons.

  1 citation

• From magnetic order to valence-change crossover in EuPd$_2$(Si$_{1-x}$Ge$_x$)$_2$ using He-gas pressure

  Bernd Wolf, Felix Spathelf, Jan Zimmermann, Theresa Lundbeck, Marius Peters, Kristin Kliemt, Cornelius Krellner, Michael Lang

  SciPost Phys. Proc. 11, 022 (2023) · published 19 June 2023 | Toggle abstract · pdf

  We present results of magnetic susceptibility and thermal expansion measurements performed on high-quality single crystals of EuPd$_2$(Si$_{1-x}$Ge$_x$)$_2$ for 0 $\leq x \leq$ 0.2 and temperatures 2 K $\leq T \leq$ 300 K. Data were taken at ambient pressure and finite He-gas pressure $p$ $\leq$ 0.5 GPa. For $x = 0$ and ambient pressure we observe a pronounced valence-change crossover centred around $T'_V$ $\approx$ 160 K with a non-magnetic ground state. This valence-change crossover is characterized by an extraordinarily strong pressure dependence of d$T'_V$ /d$p$ = (80 $\pm 10)$ K/GPa. We observe a shift of $T'_V$ to lower temperatures with increasing Ge-concentration, reaching $T'_V$ $\approx$ 90 K for $x = 0.1$, while still showing a non-magnetic ground state. Remarkably, on further increasing $x$ to 0.2 we find a stable Eu$^{(2+\delta)+}$ valence with long-range antiferromagnetic order below $T_N$ = (47.5 $\pm$ 0.1) K, reflecting a close competition between two energy scales in this system. In fact, by the application of hydrostatic pressure as small as 0.1 GPa, the ground state of this system can be changed from long-range antiferromagnetic order for $p$ $<$ 0.1 GPa to an intermediate-valence state for $p$ $\geq$ 0.1 GPa.

  1 citation

• Magnetic properties of a multicomponent intermetallic compound Tb$_{0.25}$Dy$_{0.25}$Ho$_{0.25}$Er$_{0.25}$Al$_2$

  P. K. Jesla, Jeyaramane Arout Chelvane, R. Nirmala

  SciPost Phys. Proc. 11, 013 (2023) · published 6 June 2023 | Toggle abstract · pdf

  Polycrystalline multicomponent Laves phase rare earth intermetallic compound Tb$_{0.25}$ Dy$_{0.25}$Ho$_{0.25}$Er$_{0.25}$Al$_{2}$ has been synthesized by arc-melting and characterized by powder X-ray diffraction, magnetization and heat capacity measurements. The sample has MgCu$_2$-type cubic structure (space group Fd-3m) at 300 K. The compound Tb$_{0.25}$Dy$_{0.25}$Ho$_{0.25}$Er$_{0.25}$ Al$_{2}$ orders ferromagnetically at 50 K (T$_C$). This value is almost equal to the average of the ferromagnetic ordering temperatures of the individual RAl$_2$ (R = Tb, Dy, Ho and Er) compounds. Field dependence of magnetization below T$_C$ indicates soft-ferromagnetic nature. From the magnetization vs field data obtained near T$_C$ and the temperature dependence of heat capacity, low field magnetocaloric effect has been estimated.

  1 citation

• Sensitivity of a collisional single-atom spin probe

  Jens Nettersheim, Quentin Bouton, Daniel Adam, Artur Widera

  SciPost Phys. Core 6, 009 (2023) · published 16 February 2023 | Toggle abstract · pdf

  We study the sensitivity of a collisional single-atom probe for ultracold gases. Inelastic spin-exchange collisions map information about the gas temperature $T$ or external magnetic field $B$ onto the quantum spin-population of single-atom probes, and previous work showed enhanced sensitivity for short-time nonequilibrium spin dynamics [Phys. Rev. X 10, 011018 (2020)]. Here, we numerically investigate the steady-state sensitivity of such single-atom probes to various observables. We find that the probe shows distinct sensitivity maxima in the ($B,T$) parameter diagram, although the underlying spin-exchange rates scale monotonically with temperature and magnetic field. In parameter space, the probe generally has the largest sensitivity when sensing the energy ratio between thermal energy and Zeeman energy in an externally applied magnetic field, while the sensitivity to the absolute energy, i.e., the sum of kinetic and Zeeman energy, is low. We identify the parameters yielding sensitivity maxima for a given absolute energy, which we can relate to a direct comparison of the thermal Maxwell-Boltzmann distribution with the Zeeman-energy splitting. We compare our equilibrium results to nonequilibrium experimental results from a single-atom quantum probe, showing that the sensitivity maxima in parameter space qualitatively prevail also in the nonequilibrium dynamics, while a quantitative difference remains. Our work thereby offers a microscopic explanation for the properties and performance of this single-atom quantum probe, connecting thermodynamic properties to microscopic interaction mechanisms. Our results pave the way for optimization of quantum-probe applications in ($B,T$) parameter space beyond the previously shown boost by nonequilibrium dynamics.

  1 citation

• Delocalized states in three-terminal superconductor-semiconductor nanowire devices

  P. Yu, B. D. Woods, J. Chen, G. Badawy, E. P. A. M. Bakkers, T. D. Stanescu, S. M. Frolov

  SciPost Phys. 15, 005 (2023) · published 11 July 2023 | Toggle abstract · pdf

  We fabricate three-terminal hybrid devices consisting of a semiconductor nanowire segment proximitized by a grounded superconductor and having tunnel probe contacts on both sides. By performing simultaneous tunneling measurements, we identify delocalized states, which can be observed from both ends, and states localized near one of the tunnel barriers. The delocalized states can be traced from zero magnetic field to fields beyond 0.5 T. Within the regime that supports delocalized states, we search for correlated low-energy features consistent with the presence of Majorana zero modes. While both sides of the device exhibit ubiquitous low-energy features at high fields, no correlation is inferred. Simulations using a one-dimensional effective model suggest that the delocalized states, which extend throughout the whole system, have large characteristic wave vectors, while the lower momentum states expected to give rise to Majorana physics are localized by disorder. To avoid such localization and realize Majorana zero modes, disorder needs to be reduced significantly. We propose a method for estimating the disorder strength based on analyzing the level spacing between delocalized states.

  1 citation

• Optomechanical damping as the origin of sideband asymmetry

  João D. P. Machado, Yaroslav M. Blanter

  SciPost Phys. Core 5, 034 (2022) · published 23 June 2022 | Toggle abstract · pdf

  Sideband asymmetry in cavity optomechanics has been explained by particle creation and annihilation processes, which bestow an amplitude proportional to 'n+1' and 'n' excitations to each of the respective sidebands. We discuss the issues with this as well as other interpretations, such as quantum backaction and noise interference, and show that the asymmetry is due to the optomechanical damping caused by the probe and the cooling lasers instead.

  1 citation

• From classical to quantum regime of topological surface states via defect engineering

  Maryam Salehi, Xiong Yao, Seongshik Oh

  SciPost Phys. Lect. Notes 58 (2022) · published 21 July 2022 | Toggle abstract · pdf

  Since the notion of topological insulator (TI) was envisioned in late 2000s, topology has become a new paradigm in condensed matter physics. Realization of topology as a generic property of materials has led to numerous predictions of topological effects. Although most of the classical topological effects, directly resulting from the presence of the spin-momentum-locked topological surface states (TSS), were experimentally confirmed soon after the theoretical prediction of TIs, many topological quantum effects remained elusive for a long while. It turns out that native defects, particularly interfacial defects, have been the main culprit behind this impasse. Even after quantum regime is achieved for the bulk states, TSS still tends to remain in the classical regime due to high density of interfacial defects, which frequently donate mobile carriers due to the very nature of the topologically-protected surface states. However, with several defect engineering schemes that suppress these effects, a series of topological quantum effects have emerged including quantum anomalous Hall effect, quantum Hall effect, quantized Faraday/Kerr rotations, topological quantum phase transitions, axion insulating state, zeroth-Landau level state, etc. Here, we review how these defect engineering schemes have allowed topological surface states to pull out of the murky classical regime and reveal their elusive quantum signatures, over the past decade.

  1 citation

• Anisotropic Zeeman Splitting in YbNi4P2

  Sara Karbassi, Saman Ghannadzadeh, Kristin Kliemt, Manuel Brando, Cornelius Krellner, Sven Friedemann

  SciPost Phys. 5, 056 (2018) · published 30 November 2018 | Toggle abstract · pdf

  The electronic structure of heavy-fermion materials is highly renormalised at low temperatures with localised moments contributing to the electronic excitation spectrum via the Kondo effect. Thus, heavy-fermion materials are very susceptible to Lifshitz transitions due to the small effective Fermi energy arising on parts of the renormalised Fermi surface. Here, we study Lifshitz transitions that have been discovered in YbNi4P2 in high magnetic fields. We measure the angular dependence of the critical fields necessary to induce a number of Lifshitz transitions and find it to follow a simple Zeeman-shift model with anisotropic g-factor. This highlights the coherent nature of the heavy quasiparticles forming a renormalised Fermi surface. We extract information on the orientation of the Fermi surface parts giving rise to the Lifshitz transitions and we determine the anisotropy of the effective g-factor to be $\eta \approx 3.8$ in good agreement with the crystal field scheme of YbNi4P2.