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Quantum transport theory for unconventional magnets; interplay of altermagnetism and p-wave magnetism with superconductivity
by Tim Kokkeler, Ilya Tokatly, F. Sebastian Bergeret
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Submission summary
Authors (as registered SciPost users): | F. Sebastian Bergeret · Tim Kokkeler · Ilya Tokatly |
Submission information | |
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Preprint Link: | https://arxiv.org/abs/2412.10236v1 (pdf) |
Date submitted: | 2025-01-29 13:23 |
Submitted by: | Kokkeler, Tim |
Submitted to: | SciPost Physics |
Ontological classification | |
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Academic field: | Physics |
Specialties: |
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Approaches: | Theoretical, Phenomenological |
Abstract
We present a quantum transport theory for generic magnetic metals, in which magnetism occurs predominantly due to exchange interactions, such as ferromagnets, antiferromagnets, altermagnets and p-wave magnets. Our theory is valid both for the normal and the superconducting state. We derive the effective low-energy action for each of these materials, where the spin space groups are used to determine the form of the tensor coefficients appearing in the action. The transport equations, which are obtained as the saddle point equations of this action, describe a wider range of phenomena than the usual quasiclassical equations. In ferromagnets, in addition to the usual exchange field and spin relaxation effects, we identify a spin-dependent renormalization of the diffusion coefficient, which provides a description of spinpolarized currents in both the normal and superconducting equal spin-triplet states. In the normal state, our equations provide a complete description of the spin-splitting effect in diffusive systems, recently predicted in ideal clean altermagnets. In the superconducting state, our equations predict a proximity induced magnetization, the appearance of a spontaneous magnetic moment in hybrid superconductor-altermagnet systems. The distribution and polarization direction of this magnetic moment depend on the symmetry of the structure, thus measurements of such polarization reveal the underlying microscopic symmetry of the altermagnet. Finally, for inversionsymmetry broken antiferromagnets, such as the p-wave magnet, we show that spin-galvanic effects which are distinguishable from the spin-galvanic effect induced by spin-orbit coupling only in the superconducting state. Besides these examples, our model applies to arbitrary magnetic systems, providing a complete theory for nonequilibrium transport in diffusive nonconventional magnets at arbitrary temperatures.
Author indications on fulfilling journal expectations
- Provide a novel and synergetic link between different research areas.
- Open a new pathway in an existing or a new research direction, with clear potential for multi-pronged follow-up work
- Detail a groundbreaking theoretical/experimental/computational discovery
- Present a breakthrough on a previously-identified and long-standing research stumbling block
Current status:
Reports on this Submission
Strengths
This paper discusses very current topic about altermagnet / superconductor junctions. They presented a general and reasonable theoretical scheme and predicted very interesting quantum phenomena.
Report
In this paper, the authors have presented the quasiclassical transport theory for materials with magnetic exchange and superconducting correlations. Starting from the Keldysh nonlinear sigma model, they have derived effective low-energy action based on spin space group and transport equations, which are obtained as the saddle point equations of this action. Their theory is very generic and useful for the study of ferromagnet junctions including altermagnet and p-wave magnet. They have predicted spontaneous magnetic moments in superconductor / altermagnet junction and spin-galvanic effect in p-wave magnet junctions. Since studying these unconventional magnets is a current hot topic now, the obtained formulation and results in superconductor / unconventional magnet junction are really timely and exciting. Thus, I appreciate this paper and recommend publication. Before publication, I would like to ask the authors to consider the following points.
1. It is better to explain physically why eq. (10) is obtained.
2. Please check eq. (15) again.
3. I would like to ask about the magnitude of magnetic order. To be consistent with quasiclassical theory, it is much smaller and should be the same order of the pair potential of superconductors. Is it true?
4. The authors have discussed the spin-triplet pairing in various places in superconductor / magnet junctions. Since magnets are diffusive, I think the resulting spin-triplet pairing should be odd-frequency. Is it really true? Since odd-frequency pairing has been studied up to now in superconducting junctions (Refs. Rev. Mod. Phys. 77, 1321, 2005, J. Phys. Soc. Jpn. 81, 011013, 2012). The discussion about the odd-frequency pairing is appreciated.
5. Below eq. (82), it is written that “there is an intermediate angle for which the anomalous current vanishes.” Can you predict the intermediate angle?
6. How about the condition of anomalous current appears? Is it the case both the time reversal symmetry and spatial inversion symmetry are broken?
7. Below eq. (86), there is a discussion about the p-wave magnet with homogeneous superconductor. There is a relevant work in arXiv:2501.08646.
Recommendation
Publish (surpasses expectations and criteria for this Journal; among top 10%)
Report
In this work, the authors introduce a unified framework to describe the transport of itinerant spin and charge across a magnetic conductor in both normal and superconducting states. This framework is based on the extension of the Keldysh non-linear sigma model (KNLSM) for disordered electrons to magnetic conductors, where the thermal average of the order parameter corresponds to the Green function of the electron fluid. The particular functional form of the action is determined, beyond the KNLSM, from (spin-group) symmetry considerations, and its saddle-point equations represent a generalization of the Usadel equations for the superconducting state, whose validity holds in a wide range of temperatures (far from the critical point). The authors apply their general framework to different classes of magnetic materials, such as ferromagnets and antiferromagnets (conventional magnetism), as well as altermagnets and p-wave magnets (unconventional magnetism), and they predict exciting new physics in both normal and superconducting phases.
The results obtained here are very interesting as well as timely, and the physics/methodology discussed seems overall correct. That being said, I would like to raise the following concerns/comments:
1- In Eq, (3), does the τ3 multiply ξa instead of ξs?
2- Throughout the text, the authors refer to ϕ as the superconducting phase, but in the formulas it reads φ.
3- In Eq. (22), there is a matrix σa missing in the term parametrized by the tensor χ
4- Why are Eqs. (23), (59) and (84) different? The superconducting term is either absent or have different forms in the first commutator of the right-hand side of the equation.
5- Does the minus sign in Eq. (32) only affects the first term g∂kg? If this equation is derived from Eq. (24), it should be like this. The same applies to Eqs. (60) and (85).
6- The authors should provide a reference (or a derivation in the appendices) for Eq. (34).
7- I have found a discrepancy between Eqs. (42)-(43) and (45)-(46) if Eq. (44) is correct. Is there a factor 2 missing in the term γP of Eq. (44)? In addition, does P in this equation refer to Pz?
8- The authors should provide a reference for Eq. (47).
9- In Eq. (48), what is the definition of ˜f? I think that it is provided in Eq. (F6), but it should be also given in the main text.
10- a) In Eqs. (53) and (54), should ˜f be replaced by f in the first two terms of the right-hand side?
b) Should it read ∂x˜f↓↓ in the second term of the right-hand side?.
c) What is the value of/expression for σ in these equations?
11- In Eq. (56), it should read j(−h)∗ instead of J(−h)∗
12- According to Eqs. (28) and (29), D should not be a global prefactor in Eq. (60). The same applies to Eq. (61) for the torque and to Eq. (85) for the current.
13- In the subsection ‘Superconductivity and altermagnets’, how are fs and ft related to f0 and fz introduced after Eq. (49)?. If they are the same, I would recommend the authors to unify the notation.
14- In Eqs. (67) and (68), there is a −D prefactor missing in front of the ∂xf terms (see comment #12). In addition, which component of the polarization axis does Pa refer to?
15- After Eq. (69), what does qk refer to? Is it the superconducting phase gradient q?
16- Again, which component does Pa refer to in Eq. (72)? The left-hand side of this equation represents a scalar, whereas the right-hand side represents a vector (indexed by a).
17- In Eq, (74), what does γB mean? The Kuprianov-Lukichev boundary conditions are formally introduced in Appendix G and no discussion of them is found in the main text.
18- In Eqs. (73)—(80) there are issues with the global prefactor D and the value of Pa along the lines of comments #12 and #16
19- In Eq. (87), the prefactor of the second term should read (1−σz)
20- In Eq. A15, the third term should contain τ3σyσaσy instead of τ3σaσyσaσy. The same applies to the third term of Eq. (A19).
21- After Eq. (A20), I guess that the authors mean that the tensors are even/odd in spin indices.
22- In Eq. (B7), there are subindices ‘j’ missing in the partial derivatives of Q appearing in the functional derivatives of the action.
23- How are Eqs. (C3)-(C5) related to Eqs. (50)-(52)?
For example, there is a prefactor 2 appearing on the right-hand side of Eqs. (C3)-(C5) that is not present in Eqs. (50)-(52).
24- What is the definition of hm and ˜h in Eqs. (C3)-(C5)?
25- After Eq. (C9), is the expression for the superconducting coherence length ξ correct? (for example, P⟶γP?)
26- In Eq. (C10), which is the effect of the conductivities σ↑, σ↓ [see Eq. (53)]?
27- Similar to the comment #12, in Eqs. (E1)—(E4) there are issues with the global prefactor D and the use of the tensors T and K.
28- Before Eq. (E20) and in Eq. (E21), the boundary condition should be applied at y=±Ly/2, not at z=±Ly/2
29- In Eq. (E20) should it read σD instead of D?
30- The right-hand side of Eq. (E24) should read (1/ls)2μsz
31- Unify the subindex of λ in Eqs. (E38) and (E39).
32- Check the global prefactor D in Eqs. (F10)—(F13)
33- Are there terms missing in Eq. (F27)?
I would recommend the publication of this manuscript in SciPost Physics if the authors address the above concerns satisfactorily.
Recommendation
Ask for major revision
Author: Tim Kokkeler on 2025-04-23 [id 5404]
(in reply to Report 1 on 2025-03-14)We thank the Referee for their assessment of our manuscript and the useful comments. We have included our response in the attachment.
Author: Tim Kokkeler on 2025-04-23 [id 5405]
(in reply to Report 2 on 2025-04-16)We thank the Referee for their assessment of our manuscript and the useful comments. In the attached file we provide our response to the points raised by the Referee.
Attachment:
Referee_2_response.pdf