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Muonium reaction in MgO: A showcase for the final steps of ion implantation

by Rui C. Vilão, Ali Roonkiani, Apostolos G. Marinopoulos, Helena V. Alberto, João M. Gil, Ricardo B. L. Vieira, Robert Scheuermann and Alois Weidinger

This Submission thread is now published as

Submission summary

Authors (as registered SciPost users): Apostolos Marinopoulos · Rui Vilão
Submission information
Preprint Link: scipost_202504_00035v3  (pdf)
Date accepted: Aug. 4, 2025
Date submitted: July 23, 2025, 11:57 a.m.
Submitted by: Rui Vilão
Submitted to: SciPost Physics
Ontological classification
Academic field: Physics
Specialties:
  • Condensed Matter Physics - Experiment
Approaches: Theoretical, Experimental

Abstract

We present an in-depth investigation of the implantation of positive muons in magnesium oxide (MgO). Muonium, the positive muon plus an electron is an analogue of the hydrogen atom. This study describes the final stage of the implantation process, from muon diffusion over the potential barrier and the stopping by an inelastic reaction to the final embedding of the muon into the lattice structure. A special aspect is a relatively long-lived intermediate configuration which lasts for several hundred nanoseconds or more and is accessible to muon spin spectroscopy. The model presented here provides a framework for the analysis of the general case of ion implantation.

Author indications on fulfilling journal expectations

  • Provide a novel and synergetic link between different research areas.
  • Open a new pathway in an existing or a new research direction, with clear potential for multi-pronged follow-up work
  • Detail a groundbreaking theoretical/experimental/computational discovery
  • Present a breakthrough on a previously-identified and long-standing research stumbling block

Author comments upon resubmission

We resubmit our manuscript after taking into account the comments of the referees.

List of changes

As a reply to the comments of referees 1 and 3, we have corrected the references and changed the first paragraph of the introduction.

Published as SciPost Phys. Core 8, 056 (2025)


Reports on this Submission

Report #2 by Jess Brewer (Referee 3) on 2025-7-30 (Invited Report)

  • Cite as: Jess Brewer, Report on arXiv:scipost_202504_00035v3, delivered 2025-07-30, doi: 10.21468/SciPost.Report.11671

Strengths

  1. Substantial and thorough measurements of muSR spectra in the sample.
  2. Sophisticated use of DFT calculations to determine muon & muonium sites and lattice responses.
  3. Ingenious deployment of a toy model.

Weaknesses

  1. Electric field measurements that conflict with the model are ignored completely.
  2. Unshakeable faith in a toy model.

Report

I would like to see this paper published, because it seems that only a general scientific consensus will have any effect on the authors' convictions.

Requested changes

None at this point.

Attachment


Recommendation

Publish (easily meets expectations and criteria for this Journal; among top 50%)

  • validity: low
  • significance: high
  • originality: top
  • clarity: good
  • formatting: good
  • grammar: good

Report #1 by Anonymous (Referee 4) on 2025-7-24 (Invited Report)

  • Cite as: Anonymous, Report on arXiv:scipost_202504_00035v3, delivered 2025-07-24, doi: 10.21468/SciPost.Report.11628

Report

I insist that the manuscript lacks crucial experiments which are absolutely necessary to set an experimental basis before suggesting any model. In their reply to my previous comments the authors presented no argumentation against my suggestions.
The model itself does not stand critics expressed in Phys. Rev. B 101, 077201 (2020), in particular, regarding timescales and energies involved.

Recommendation

Reject

  • validity: low
  • significance: good
  • originality: poor
  • clarity: ok
  • formatting: reasonable
  • grammar: good

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Comments

Anonymous on 2025-07-30  [id 5694]

The "anonymous" Referee is obviously one of my coauthors on the critique paper Phys. Rev. B 101, 077201 (2020) who is less charitable than I am regarding the intransigence of Vilao et al. My position is that the authors of the current paper should be given all the rope they need to hang themselves in public, but I have a lot of sympathy for my own coauthors: Vilao et al. have again systematically ignored the results of our electric field experiments, presumably because those results are incompatible with their "transition state" (a.k.a. "doorway state") model. I mention all this because I am sorely tempted to just agree with the other Referee and reject this paper, but I feel more obliged to acknowledge the ingenuity of their model and the detailed experiments they have done this time, and leave the ultimate evaluation to general scientific consensus, which requires publication. Ultimately, the hard decision is in the Editor's hands.