TY  - JOUR
PB  - SciPost Foundation
DO  - 10.21468/SciPostPhys.15.4.138
TI  - Photon pumping, photodissociation and dissipation at interplay for the fluorescence of a molecule in a cavity
PY  - 2023/10/05
UR  - https://scipost.org/SciPostPhys.15.4.138
JF  - SciPost Physics
JA  - SciPost Phys.
VL  - 15
IS  - 4
SP  - 138
A1  - Gopalakrishna, Megha
AU  - Viñas Boström, Emil
AU  - Verdozzi, Claudio
AB  - We introduce a model description of a diatomic molecule in an optical cavity, with pump and fluorescent fields, and electron and nuclear motion are treated on equal footing and exactly. The model accounts for several optical response temporal scenarios: A Mollow spectrum hindered by electron correlations, a competition of harmonic generation and molecular dissociation, a dependence of fluorescence on photon pumping rate and dissipation. It is thus a general and flexible template for insight into experiments where quantum photon confinement, leakage, nuclear motion and electronic correlations are at interplay.
ER  -

@Article{10.21468/SciPostPhys.15.4.138,
	title={{Photon pumping, photodissociation and dissipation at interplay for the fluorescence of a molecule in a cavity}},
	author={Megha Gopalakrishna and Emil Viñas Boström and Claudio Verdozzi},
	journal={SciPost Phys.},
	volume={15},
	pages={138},
	year={2023},
	publisher={SciPost},
	doi={10.21468/SciPostPhys.15.4.138},
	url={https://scipost.org/10.21468/SciPostPhys.15.4.138},
}