Publications

Order by: publication date number of citations

• Pressure-dependent structural and electronic instabilities in LaSb$_2$

  Theodore I. Weinberger, Christian K. de Podesta, Jiasheng Chen, Stephen A. Hodgson, F. Malte Grosche

  SciPost Phys. Proc. 11, 018 (2023) · published 6 June 2023 | Toggle abstract · pdf

  LaSb$_2$ exhibits a large, non-saturating, linear magnetoresistance at low temperatures, defying the expectations of Fermi liquid theory. This is thought to be caused by charge density wave order emerging below an abrupt, hysteretic anomaly in the resistivity at $\sim$ 355 K. We find that, under hydrostatic pressure, this anomaly becomes much more pronounced, develops strong hysteresis, and shifts rapidly towards lower temperatures. The anomaly is fully suppressed by only 6 kbar. Moreover, we observe a second transition anomaly at lower temperature, which likewise disappears under pressure. These findings are discussed in the context of a structural transition recently discovered in the sister material CeSb$_2$ and of density functional theory calculations, which indicate that the SmSb$_2$-type structure adopted by LaSb$_2$ at ambient conditions is unstable at moderate applied pressures.

  2 citations

• Local investigation of the crystal electric field ground-state in CeCu(Sb,Bi)$_2$ heavy fermions

  Davi Zau, G. S. Freitas, P. G. Pagliuso, R. R. Urbano

  SciPost Phys. Proc. 11, 017 (2023) · published 6 June 2023 | Toggle abstract · pdf

  In this work, we performed systematic Nuclear Magnetic Resonance (NMR) and magnetic susceptibility experiments in CeCuSb$_2$ single-crystals. The main findings were compared to previous report for CeCuBi$_2$. The NMR spectra and transferred hyperfine coupling for the $^{63}$Cu nuclei were obtained aiming to observe their correlation with the crystal electric field (CEF) effects on the Ce$^{3+}$ ($J=5/2$) multiplet. Besides, in an attempt to elucidate the magnetic structure through NMR measurements at different magnetic fields orientations, we observed a magnetic transition at $T\approx 8\,$K higher than the Néel temperature $T_N$ measured by magnetic susceptibility indicating the development of short-range magnetic ordering above T$_N$. In addition, the wipe out of the main NMR resonance line and a persistent spin-echo signal throughout the whole frequency-swept range suggest the possibility of an incommensurate magnetic structure in CeCuSb$_2$. Furthermore, the small transferred hyperfine coupling constant found for CeCuSb$_2$ indicates a scenario with more localized Ce$^{3+}$ 4f electrons than for CeMIn$_5$ (M $=$ Co,Rh,Ir) heavy fermions family. Additionally, subtle changes in the hybridization between the $^{63}$Cu with the 4f$^1$ Ce$^{3+}$ electrons in distinct magnetic field orientations allowed us to provide detailed information and map out the 4f CEF orbital ground-state of CeCu(Sb,Bi)$_2$ via NMR measurements.

• EPR and SQUID interrogations of Cr(III) trimer complexes in the MIL-101(Cr) and bimetallic MIL-100(Al/Cr) MOFs

  Kavipriya Thangavel, Andrea Folli, Michael Ziese, Steffen Hausdorf, Stefan Kaskel, Damien M. Murphy, Andreas Pöppl

  SciPost Phys. Proc. 11, 016 (2023) · published 6 June 2023 | Toggle abstract · pdf

  Herein, electron paramagnetic resonance (EPR) spectroscopy at X- (9.4 GHz), Q- (34 GHz) and W-band (95 GHz), and superconducting quantum interference device (SQUID) measurements on antiferromagnetically coupled metal trimers in MIL-101(Cr) and MIL-100(Al$_{0.8}$Cr$_{0.2}$) MOFs were investigated. At low temperatures, the Cr(III) trimers exhibit a Dzyaloshinsky-Moriya (D-M) interaction, and have a total spin state S$_T = 1/2$.

• Field-induced local Fermi-liquid states in the underscreened Kondo model for Eu compounds

  Shingo Kuniyoshi, Ryousuke Shiina

  SciPost Phys. Proc. 11, 015 (2023) · published 6 June 2023 | Toggle abstract · pdf

  We have studied an underscreened Kondo model for the impurity spin $S=7/2$ capturing the $4f$ characteristics of a nearly divalent Eu ion. By using the numerical renormalization group method, it is shown that an unusual heavy-fermion state is induced from the underscreened spin state when a weak crystal field is introduced. It is also found that the application of the magnetic field enhances the effective mass of the heavy fermions, reflecting the field-induced level crossing of the spin states. We will discuss the mechanism of these mass enhancements in terms of a realization of the two-stage Kondo effect.

• Josephson effects between the Kitaev ladder superconductors

  Osamu Kanehira, Hiroki Tsuchiura

  SciPost Phys. Proc. 11, 014 (2023) · published 6 June 2023 | Toggle abstract · pdf

  The two-leg ladder system consisting of the Kitaev chains is known to exhibit a richer phase diagram than that of the single chain. We theoretically investigate the variety of the Josephson effects between the ladder systems. We consider the Josephson phase difference $\theta$ between these two ladder systems as well as the phase difference $\phi$ between the parallel chains in each ladder system. The total energy of the junction at $T = 0$ is calculated by a numerical diagonalization method as functions of $\theta$, $\phi$, and also a transverse hopping $t_{\perp}$ in the ladders. We find that, by controlling $t_{\perp}$ and $\phi$, the junction exhibits not only the fractional Josephson effect for the phase difference $\theta$, but also the usual 0-junction and even $\pi$-junction properties.

• Magnetic properties of a multicomponent intermetallic compound Tb$_{0.25}$Dy$_{0.25}$Ho$_{0.25}$Er$_{0.25}$Al$_2$

  P. K. Jesla, Jeyaramane Arout Chelvane, R. Nirmala

  SciPost Phys. Proc. 11, 013 (2023) · published 6 June 2023 | Toggle abstract · pdf

  Polycrystalline multicomponent Laves phase rare earth intermetallic compound Tb$_{0.25}$ Dy$_{0.25}$Ho$_{0.25}$Er$_{0.25}$Al$_{2}$ has been synthesized by arc-melting and characterized by powder X-ray diffraction, magnetization and heat capacity measurements. The sample has MgCu$_2$-type cubic structure (space group Fd-3m) at 300 K. The compound Tb$_{0.25}$Dy$_{0.25}$Ho$_{0.25}$Er$_{0.25}$ Al$_{2}$ orders ferromagnetically at 50 K (T$_C$). This value is almost equal to the average of the ferromagnetic ordering temperatures of the individual RAl$_2$ (R = Tb, Dy, Ho and Er) compounds. Field dependence of magnetization below T$_C$ indicates soft-ferromagnetic nature. From the magnetization vs field data obtained near T$_C$ and the temperature dependence of heat capacity, low field magnetocaloric effect has been estimated.

  1 citation

• High field magnetism of the triangular lattice antiferromagnet CsFeCl$_3$ under high pressure

  Katsuki Nihongi, Takanori Kida, Yasuo Narumi, Nobuyuki Kurita, Hidekazu Tanaka, Yoshiya Uwatoko, Koichi Kindo, Masayuki Hagiwara

  SciPost Phys. Proc. 11, 012 (2023) · published 5 June 2023 | Toggle abstract · pdf

  Magnetization measurements of the triangular lattice antiferromagnet CsFeCl$_{3}$ at 1.4 K for $H \parallel c$ were performed in pulsed high magnetic fields of up to 51 T under high pressures of up to 0.80 GPa. At ambient pressure, the magnetization below $H_{\rm c1}$ = 4 T is small, and then it changes steeply between $H_{\rm c1}$ and $H_{\rm c2}$ = 12 T, followed by a gradual increase in magnetization up to $H_{\rm m}$ = 33 T where a two-step metamagnetic transition occurs. With increasing pressure, the $H_{\rm c1}$ and $H_{\rm m}$ shifted to the low-field side, while the $H_{\rm c2}$ shifted to the opposite side. The change in $H_{\rm m}$ may depend on the difference in the single-ion anisotropies on pressure in the lowest $J$ = 1 and the excited $J$ = 2 states.

• Correlation between antiferromagnetic and charge-density-wave order in UPt$_{2}$Si$_{2}$ studied by resonant X-Ray scattering

  Fusako Kon, Chihiro Tabata, Kodai Miura, Ruo Hibino, Hiroyuki Hidaka, Tatsuya Yanagisawa, Hironori Nakao, Hiroshi Amitsuka

  SciPost Phys. Proc. 11, 011 (2023) · published 5 June 2023 | Toggle abstract · pdf

  Relationship between antiferromagnetic order with Néel temperature of 35 K and charge-density-wave (CDW) order below 320 K of UPt$_2$Si$_2$ has been investigated by resonant X-ray scattering measurements. We have found that a resonant scattering signal develops below the Néel temperature at the ${ M}_{ 4}$ absorption edge of uranium with a propagation vector of the CDW order ${ q}_{ CDW} \sim$ (0.42, 0, 0). The experimental results reveal that the magnetic structure of UPt$_2$Si$_2$ is modulated by the CDW ordering.

  2 citations

• Transport and magnetic properties in the Nd diluted system Y$_{1-x}$Nd$_{x}$Co$_{2}$Zn$_{20}$

  Rikako Yamamoto, Yasuyuki Shimura, Kazunori Umeo, Toshiro Takabatake, Takahiro Onimaru

  SciPost Phys. Proc. 11, 010 (2023) · published 5 June 2023 | Toggle abstract · pdf

  We report the electrical resistivity, specific heat, and magnetization measurements of Y$_{1-x}$Nd$_{x}$Co$_{2}$Zn$_{20}$ for $0.017 \leq x \leq 0.95$. The Schottky-type specific heat peak at around 13 K for all the samples is reproduced by the crystalline electric field model with the $\Gamma_{6}$ doublet ground state of a Nd$^{3+}$ ion. The magnetization and magnetic susceptibility data of the samples for $x \leq 0.06$ are well reproduced by the calculation without intersite magnetic interactions among Nd moments. Therefore, the dilute Nd system Y$_{1-x}$Nd$_{x}$Co$_{2}$Zn$_{20}$ for $x \leq 0.06$ is a good candidate to study on-site interaction of the $\Gamma_{6}$ doublet ground state of 4$f$ electrons with conduction electrons.

  1 citation

• Photoinduced pairing in Mott insulators

  Satoshi Ejima, Holger Fehske

  SciPost Phys. Proc. 11, 009 (2023) · published 5 June 2023 | Toggle abstract · pdf

  Utilizing time-evolution techniques in (infinite) matrix-product-state representation, we study the non-equilibrium dynamics of driven Mott insulators and demonstrate photoinduced $\eta$ pairing directly in the thermodynamic limit. Analyzing the time evolution of the corresponding pairing correlations, we determine the optimal laser pump parameters for which long-range $\eta$-pairing becomes dominant after pulse irradiation. The time-dependent photoemission spectra for this optimal pump parameter set show clear signatures of the photoinduced insulator-to-metal phase transition related to the formation of $\eta$ pairs.