Non-collinear magnetic structures in the magnetoelectric Swedenborgite CaBaFe4O7 derived by powder and single-crystal neutron diffraction
N. Qureshi, B. Ouladdiaf, A. Senyshyn, V. Caignaert, M. Valldor
SciPost Phys. Core 5, 007 (2022) · published 3 February 2022
- doi: 10.21468/SciPostPhysCore.5.1.007
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Abstract
We have investigated the magnetic structures of the Swedenborgite compound CaBaFe4O7 using magnetic susceptibility and neutron diffraction experiments on powder and single-crystal samples. Below TN1 = 274 K the system orders in a ferrimagnetic structure with spins along the c axis and an additional antiferromagnetic component within the kagome plane which obviously cannot satisfy all exchange interactions. Competing single-ion anisotropy and exchange interactions lead to a transition into a multi-q conical structure at TN2 = 202 K. The derivation of the complex ordering scheme below TN2 is an important step towards the understanding of the magnetoelectric effect under magnetic fields in this polar ferrimagnet.
Cited by 2
Authors / Affiliations: mappings to Contributors and Organizations
See all Organizations.- 1 2 Navid Qureshi,
- 2 Bachir Ouladdiaf,
- 3 Anatoliy Senyshyn,
- 4 Vincent Caignaert,
- 1 5 Martin Björn Valldor
- 1 Universität zu Köln / University of Cologne [UoC]
- 2 Institut Laue-Langevin [ILL]
- 3 Technische Universität München / Technical University of Munich [TUM]
- 4 Laboratoire de Cristallographie et Sciences des Matériaux [CRISMAT]
- 5 Universitetet i Oslo / University of Oslo [UiO]