SciPost Physics Proceedings

SciPost Physics Proceedings issue 11

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• Quantum spin nematic liquid in the low-dimensional anisotropic magnets -S=1/2 delta spin chain with the anisotropic ferromagnetic interaction in magnetic field-

  Toru Sakai, Rito Furuchi, Hiroki Nakano, Kiyomi Okamoto

  SciPost Phys. Proc. 11, 001 (2023) · published 5 June 2023 | Toggle abstract · pdf

  The magnetization process of the $S=1/2$ delta chain with the anisotropic ferromagnetic interaction is investigated using the numerical diagonalization of finite-size clusters. It is found that the spin nematic liquid phase appears in higher magnetization region, as well as the SDW liquid one in lower region.

• Single crystal growth of PrNiGe$_2$ compounds

  Kousei Ishiwatari, Kaito Hoshii, Keisuke Ida, Masashi Ohashi

  SciPost Phys. Proc. 11, 002 (2023) · published 5 June 2023 | Toggle abstract · pdf

  We report on the magnetic characterization of a praseodym intermetallic PrNiGe$_2$. Several single crystals are grown by the Czochralski method from Ni- deficient sample as the initial one. X-ray analysis of PrNi$_{0.8}$Ge$_2$ indicated the CeNiSi$_2$-type structure as the only phase. The magnetic measurements clearly indicate that PrNi$_x$Ge$_2$ exhibits a ferromagnetic orderings at 12 K, which is independent with of composition of Ni. A strong anisotropy along the three principal crystallographic directions was observed, reflecting the orthorhombic symmetry of the crystal structure. The $b$-axis was found to be the easy axis of magnetization.

• Efficient scheme for time-dependent thermal pure quantum state: Application to the Kitaev model with armchair edges

  Hirokazu Taguchi, Akihisa Koga, Yuta Murakami

  SciPost Phys. Proc. 11, 003 (2023) · published 5 June 2023 | Toggle abstract · pdf

  We consider the time-dependent thermal pure quantum state method and introduce the efficient scheme to evaluate the change in physical quantities induced by the time-dependent perturbations, which has been proposed in our previous paper [H. Taguchi et al., Phys. Rev. B 105, 125137 (2022)]. Here, we treat the Kitaev model to consider the Majorana-mediated spin transport, as an example. We demonstrate how efficient our scheme is to evaluate spin oscillations induced by the magnetic field pulse.

• A testable theory for high-Tc superconductivity in cuprates

  Eduardo C. Marino

  SciPost Phys. Proc. 11, 004 (2023) · published 5 June 2023 | Toggle abstract · pdf

  A number of theories for the superconductivity in cuprates, have been proposed in the more than 30 years that have elapsed since its discovery. A common feature of these theories is the small number, or even the absence, of quantitative predictions that could be compared to a vast number of experimental data, which are, conversely, available. Such theories are, consequently non-testable. We describe the foundations and a number of applications of a theory describing High-Tc Superconductivity in cuprates, which we proposed recently, that besides being testable, has proven to meet successfully the tests to which it has been submitted so far.

• Magnetic properties of the putative higher-order topological insulator EuIn$_2$As$_2$

  Tomasz Toliński, Dariusz Kaczorowski

  SciPost Phys. Proc. 11, 005 (2023) · published 5 June 2023 | Toggle abstract · pdf

  In higher-order topological insulator (HOTI), a gap is preserved both for the bulk and the surface states, and only hinges or corners become gapless. Recently, it has been predicted that the antiferromagnetic compound EuIn$_2$As$_2$ can host both the HOTI and axion insulator features. Preliminary experimental confirmation of this finding was obtained using angle-resolved photoemission spectroscopy. The main objective of this work was to characterize the anisotropic magnetic properties of single-crystalline EuIn$_2$As$_2$. In addition, complementary studies on the transport properties, heat capacity, and magnetocaloric effect in this compound were performed.

• Hidden-orders of uranium compounds

  Hisatomo Harima

  SciPost Phys. Proc. 11, 006 (2023) · published 5 June 2023 | Toggle abstract · pdf

  Hidden order is often discussed in strongly correlated electron systems. In many cases, it shows no magnetic responses, so that the order parameter is electric, but accompanies few lattice distortion. In the Jahn-Teller cases, the ordered state gains its energy by changing inter-site mixing strengths, leading a larger structural distortion with lowering symmetry. On the contrary, in strongly correlated electron systems, the strong intra-site Coulomb energy causes the the symmetry lowering. It is not necessary to bring the lattice distortion for lowering local site symmetry. In fact, lower symmetry of electronic state than the symmetry of the crystal structure can be found for UTe$_2$, UGe$_2$ similarly for URu$_2$Si$_2$.

• Structural and magnetic anisotropy in YBa$_2$Cu$_3$O$_7$/La$_{0.67}$Sr$_{0.33}$MnO$_3$ bilayer on SrTiO$_3$ substrate

  Ankita Singh, Ram Prakash Pandeya, Sawani Dutta, Srinivas C. Kandukuri, Kalobaran Maiti

  SciPost Phys. Proc. 11, 007 (2023) · published 5 June 2023 | Toggle abstract · pdf

  We study the magnetic properties and emergence of superconductivity in YBa$_2$Cu$_3$O$_7$ (YBCO)/ La$_{0.67}$Sr$_{0.33}$MnO$_3$ (LSMO) heterostructures. Bilayer films of superconducting layer, YBCO, and ferromagnetic layer, LSMO were grown on SrTiO$_{3}$ (STO) (001) substrate using ultrahigh vacuum Pulsed Laser Deposition system. Magnetization data at 100 K as a function of applied magnetic field shows ferromagnetic behaviour due to the LSMO layer. Cooling below 100 K leads to superconductivity in this material; the onset of superconductivity occurs at a temperature, $T_{c,SC},$ of 86 K for $H_{ext}\perp c$ (in-plane) \& 84 K for $H_{ext}||c$ (out-of-plane) under 100 Oe applied field. In-plane magnetic measurements show significant suppression of diamagnetic behaviour as compared to the out-of-plane measurements. The susceptibility signals are higher for out-of-plane direction. Such strong anisotropy in magnetism and the transition temperatures reveal complex interplay of magnetism and superconductivity in this system and calls for further study in this direction.

• Electronic structure of CeAuAl$_3$ using density functional theory

  André Deyerling, Marc A. Wilde, Christian Pfleiderer

  SciPost Phys. Proc. 11, 008 (2023) · published 5 June 2023 | Toggle abstract · pdf

  We studied the magnetic properties and electronic structure of $CeAuAl_3$ using density functional theory. This compound shows a large Sommerfeld coefficient, a Kondo temperature, ${T_K=4\,K}$ and antiferromagnetic order below ${T_N=1.1\,K}$. We calculated the magnetic groundstate of ${CeAuAl_3}$ and the magnetic anisotropy energies. Treating the 4f-electrons as localized with DFT+U we obtain a good match with the magnetic properties observed experimentally. We also report salient features of the electronic structure of ${CeAuAl_3}$, including features of the Fermi surface and associated quantum oscillatory spectra, when the 4f-electrons are treated either as localized or itinerant.

• Photoinduced pairing in Mott insulators

  Satoshi Ejima, Holger Fehske

  SciPost Phys. Proc. 11, 009 (2023) · published 5 June 2023 | Toggle abstract · pdf

  Utilizing time-evolution techniques in (infinite) matrix-product-state representation, we study the non-equilibrium dynamics of driven Mott insulators and demonstrate photoinduced $\eta$ pairing directly in the thermodynamic limit. Analyzing the time evolution of the corresponding pairing correlations, we determine the optimal laser pump parameters for which long-range $\eta$-pairing becomes dominant after pulse irradiation. The time-dependent photoemission spectra for this optimal pump parameter set show clear signatures of the photoinduced insulator-to-metal phase transition related to the formation of $\eta$ pairs.

• Transport and magnetic properties in the Nd diluted system Y$_{1-x}$Nd$_{x}$Co$_{2}$Zn$_{20}$

  Rikako Yamamoto, Yasuyuki Shimura, Kazunori Umeo, Toshiro Takabatake, Takahiro Onimaru

  SciPost Phys. Proc. 11, 010 (2023) · published 5 June 2023 | Toggle abstract · pdf

  We report the electrical resistivity, specific heat, and magnetization measurements of Y$_{1-x}$Nd$_{x}$Co$_{2}$Zn$_{20}$ for $0.017 \leq x \leq 0.95$. The Schottky-type specific heat peak at around 13 K for all the samples is reproduced by the crystalline electric field model with the $\Gamma_{6}$ doublet ground state of a Nd$^{3+}$ ion. The magnetization and magnetic susceptibility data of the samples for $x \leq 0.06$ are well reproduced by the calculation without intersite magnetic interactions among Nd moments. Therefore, the dilute Nd system Y$_{1-x}$Nd$_{x}$Co$_{2}$Zn$_{20}$ for $x \leq 0.06$ is a good candidate to study on-site interaction of the $\Gamma_{6}$ doublet ground state of 4$f$ electrons with conduction electrons.

• Correlation between antiferromagnetic and charge-density-wave order in UPt$_{2}$Si$_{2}$ studied by resonant X-Ray scattering

  Fusako Kon, Chihiro Tabata, Kodai Miura, Ruo Hibino, Hiroyuki Hidaka, Tatsuya Yanagisawa, Hironori Nakao, Hiroshi Amitsuka

  SciPost Phys. Proc. 11, 011 (2023) · published 5 June 2023 | Toggle abstract · pdf

  Relationship between antiferromagnetic order with Néel temperature of 35 K and charge-density-wave (CDW) order below 320 K of UPt$_2$Si$_2$ has been investigated by resonant X-ray scattering measurements. We have found that a resonant scattering signal develops below the Néel temperature at the ${ M}_{ 4}$ absorption edge of uranium with a propagation vector of the CDW order ${ q}_{ CDW} \sim$ (0.42, 0, 0). The experimental results reveal that the magnetic structure of UPt$_2$Si$_2$ is modulated by the CDW ordering.

• High field magnetism of the triangular lattice antiferromagnet CsFeCl$_3$ under high pressure

  Katsuki Nihongi, Takanori Kida, Yasuo Narumi, Nobuyuki Kurita, Hidekazu Tanaka, Yoshiya Uwatoko, Koichi Kindo, Masayuki Hagiwara

  SciPost Phys. Proc. 11, 012 (2023) · published 5 June 2023 | Toggle abstract · pdf

  Magnetization measurements of the triangular lattice antiferromagnet CsFeCl$_{3}$ at 1.4 K for $H \parallel c$ were performed in pulsed high magnetic fields of up to 51 T under high pressures of up to 0.80 GPa. At ambient pressure, the magnetization below $H_{\rm c1}$ = 4 T is small, and then it changes steeply between $H_{\rm c1}$ and $H_{\rm c2}$ = 12 T, followed by a gradual increase in magnetization up to $H_{\rm m}$ = 33 T where a two-step metamagnetic transition occurs. With increasing pressure, the $H_{\rm c1}$ and $H_{\rm m}$ shifted to the low-field side, while the $H_{\rm c2}$ shifted to the opposite side. The change in $H_{\rm m}$ may depend on the difference in the single-ion anisotropies on pressure in the lowest $J$ = 1 and the excited $J$ = 2 states.

• Magnetic properties of a multicomponent intermetallic compound Tb$_{0.25}$Dy$_{0.25}$Ho$_{0.25}$Er$_{0.25}$Al$_2$

  P. K. Jesla, Jeyaramane Arout Chelvane, R. Nirmala

  SciPost Phys. Proc. 11, 013 (2023) · published 6 June 2023 | Toggle abstract · pdf

  Polycrystalline multicomponent Laves phase rare earth intermetallic compound Tb$_{0.25}$ Dy$_{0.25}$Ho$_{0.25}$Er$_{0.25}$Al$_{2}$ has been synthesized by arc-melting and characterized by powder X-ray diffraction, magnetization and heat capacity measurements. The sample has MgCu$_2$-type cubic structure (space group Fd-3m) at 300 K. The compound Tb$_{0.25}$Dy$_{0.25}$Ho$_{0.25}$Er$_{0.25}$ Al$_{2}$ orders ferromagnetically at 50 K (T$_C$). This value is almost equal to the average of the ferromagnetic ordering temperatures of the individual RAl$_2$ (R = Tb, Dy, Ho and Er) compounds. Field dependence of magnetization below T$_C$ indicates soft-ferromagnetic nature. From the magnetization vs field data obtained near T$_C$ and the temperature dependence of heat capacity, low field magnetocaloric effect has been estimated.

• Josephson effects between the Kitaev ladder superconductors

  Osamu Kanehira, Hiroki Tsuchiura

  SciPost Phys. Proc. 11, 014 (2023) · published 6 June 2023 | Toggle abstract · pdf

  The two-leg ladder system consisting of the Kitaev chains is known to exhibit a richer phase diagram than that of the single chain. We theoretically investigate the variety of the Josephson effects between the ladder systems. We consider the Josephson phase difference $\theta$ between these two ladder systems as well as the phase difference $\phi$ between the parallel chains in each ladder system. The total energy of the junction at $T = 0$ is calculated by a numerical diagonalization method as functions of $\theta$, $\phi$, and also a transverse hopping $t_{\perp}$ in the ladders. We find that, by controlling $t_{\perp}$ and $\phi$, the junction exhibits not only the fractional Josephson effect for the phase difference $\theta$, but also the usual 0-junction and even $\pi$-junction properties.

• Field-induced local Fermi-liquid states in the underscreened Kondo model for Eu compounds

  Shingo Kuniyoshi, Ryousuke Shiina

  SciPost Phys. Proc. 11, 015 (2023) · published 6 June 2023 | Toggle abstract · pdf

  We have studied an underscreened Kondo model for the impurity spin $S=7/2$ capturing the $4f$ characteristics of a nearly divalent Eu ion. By using the numerical renormalization group method, it is shown that an unusual heavy-fermion state is induced from the underscreened spin state when a weak crystal field is introduced. It is also found that the application of the magnetic field enhances the effective mass of the heavy fermions, reflecting the field-induced level crossing of the spin states. We will discuss the mechanism of these mass enhancements in terms of a realization of the two-stage Kondo effect.

• EPR and SQUID interrogations of Cr(III) trimer complexes in the MIL-101(Cr) and bimetallic MIL-100(Al/Cr) MOFs

  Kavipriya Thangavel, Andrea Folli, Michael Ziese, Steffen Hausdorf, Stefan Kaskel, Damien M. Murphy, Andreas Pöppl

  SciPost Phys. Proc. 11, 016 (2023) · published 6 June 2023 | Toggle abstract · pdf

  Herein, electron paramagnetic resonance (EPR) spectroscopy at X- (9.4 GHz), Q- (34 GHz) and W-band (95 GHz), and superconducting quantum interference device (SQUID) measurements on antiferromagnetically coupled metal trimers in MIL-101(Cr) and MIL-100(Al$_{0.8}$Cr$_{0.2}$) MOFs were investigated. At low temperatures, the Cr(III) trimers exhibit a Dzyaloshinsky-Moriya (D-M) interaction, and have a total spin state S$_T = 1/2$.

• Local investigation of the crystal electric field ground-state in CeCu(Sb,Bi)$_2$ heavy fermions

  Davi Zau, G. S. Freitas, P. G. Pagliuso, R. R. Urbano

  SciPost Phys. Proc. 11, 017 (2023) · published 6 June 2023 | Toggle abstract · pdf

  In this work, we performed systematic Nuclear Magnetic Resonance (NMR) and magnetic susceptibility experiments in CeCuSb$_2$ single-crystals. The main findings were compared to previous report for CeCuBi$_2$. The NMR spectra and transferred hyperfine coupling for the $^{63}$Cu nuclei were obtained aiming to observe their correlation with the crystal electric field (CEF) effects on the Ce$^{3+}$ ($J=5/2$) multiplet. Besides, in an attempt to elucidate the magnetic structure through NMR measurements at different magnetic fields orientations, we observed a magnetic transition at $T\approx 8\,$K higher than the Néel temperature $T_N$ measured by magnetic susceptibility indicating the development of short-range magnetic ordering above T$_N$. In addition, the wipe out of the main NMR resonance line and a persistent spin-echo signal throughout the whole frequency-swept range suggest the possibility of an incommensurate magnetic structure in CeCuSb$_2$. Furthermore, the small transferred hyperfine coupling constant found for CeCuSb$_2$ indicates a scenario with more localized Ce$^{3+}$ 4f electrons than for CeMIn$_5$ (M $=$ Co,Rh,Ir) heavy fermions family. Additionally, subtle changes in the hybridization between the $^{63}$Cu with the 4f$^1$ Ce$^{3+}$ electrons in distinct magnetic field orientations allowed us to provide detailed information and map out the 4f CEF orbital ground-state of CeCu(Sb,Bi)$_2$ via NMR measurements.

• Pressure-dependent structural and electronic instabilities in LaSb$_2$

  Theodore I. Weinberger, Christian K. de Podesta, Jiasheng Chen, Stephen A. Hodgson, F. Malte Grosche

  SciPost Phys. Proc. 11, 018 (2023) · published 6 June 2023 | Toggle abstract · pdf

  LaSb$_2$ exhibits a large, non-saturating, linear magnetoresistance at low temperatures, defying the expectations of Fermi liquid theory. This is thought to be caused by charge density wave order emerging below an abrupt, hysteretic anomaly in the resistivity at $\sim$ 355 K. We find that, under hydrostatic pressure, this anomaly becomes much more pronounced, develops strong hysteresis, and shifts rapidly towards lower temperatures. The anomaly is fully suppressed by only 6 kbar. Moreover, we observe a second transition anomaly at lower temperature, which likewise disappears under pressure. These findings are discussed in the context of a structural transition recently discovered in the sister material CeSb$_2$ and of density functional theory calculations, which indicate that the SmSb$_2$-type structure adopted by LaSb$_2$ at ambient conditions is unstable at moderate applied pressures.

• In-plane Fermi surface mapping of ZrSiS and HfSiS by de Haas-van Alphen oscillations

  Bruno Gudac, Mihovil Bosnar, Filip Orbanić, Trpimir Ivšić, Ivan Kokanović, Mario Novak

  SciPost Phys. Proc. 11, 019 (2023) · published 6 June 2023 | Toggle abstract · pdf

  We have conducted a comprehensive experimental investigation of the in-plane de Haas van Alphen quantum oscillations in ZrSiS and HfSiS and compared the results to the ab-initio calculations. We found a moderately good agreement for a set of frequencies located between 100 T and 200 T. These could be associated with extremal orbitals of the electron pockets located around the $k_z=\pm\pi/2c$ planes at the edge of the 1st Brillouin zone. In contrast, the experimentally detected low-frequency set of oscillations found around 20 T could not be reproduced by the calculations. Further refinement of the ab-initio calculation has to be conducted to fully capture all the observed features of the Fermi surface in ZrSiS and HfSiS.

• Composition dependence of the specific heat of FeSi

  Carolina Burger, Andreas Bauer, Christian Pfleiderer

  SciPost Phys. Proc. 11, 020 (2023) · published 6 June 2023 | Toggle abstract · pdf

  Recently, a high-mobility surface conduction channel and in-gap states were identified in the correlated small-gap semiconductor FeSi using electrical transport measurements and high-resolution tunneling spectroscopy. The mobility of the charge carriers in the surface channel is quantitatively reminiscent of topological insulators, but displays a lack of sensitivity to the presence of ferromagnetic impurities as studied by means of a series of single crystals with slightly different starting compositions. Here, we report measurements of the specific heat of these crystals. At low temperatures, a shallow maximum is observed in the specific heat divided by temperature. This maximum is suppressed under magnetic field, characteristic of a Schottky anomaly associated with magnetic impurities. In comparison, the height of this maximum decreases with increasing initial iron content.

• Magnetic, electronic, and structural investigation of the strongly correlated Y$_{1-x}$Sm$_{x}$Co$_5$ system

  F. Passos, D. Cornejo, G. J. Nilsen, V. Martelli, J. Larrea Jiménez

  SciPost Phys. Proc. 11, 021 (2023) · published 6 June 2023 | Toggle abstract · pdf

  SmCo$_5$ and YCo$_5$ are isostructural compounds both showing large magnetocrystalline anisotropy, where the former originates mainly from the crystal-electric field and magnetic interactions. We investigate the contribution of both interactions by partially substituting Y by Sm in as-cast polycrystalline Y$_{1-x}$Sm$_{x}$Co$_5$ (with $x$=0.00, 0.12, 0.18, 0.31, and 0.40) and measuring their structural, magnetic, and electrical properties through X-ray diffraction, magnetization, and electrical transport measurements. Our results suggest an interplay between microstructure strain in as-cast samples and the electronic and magnetic interactions.

• From magnetic order to valence-change crossover in EuPd$_2$(Si$_{1-x}$Ge$_x$)$_2$ using He-gas pressure

  Bernd Wolf, Felix Spathelf, Jan Zimmermann, Theresa Lundbeck, Marius Peters, Kristin Kliemt, Cornelius Krellner, Michael Lang

  SciPost Phys. Proc. 11, 022 (2023) · published 19 June 2023 | Toggle abstract · pdf

  We present results of magnetic susceptibility and thermal expansion measurements performed on high-quality single crystals of EuPd$_2$(Si$_{1-x}$Ge$_x$)$_2$ for 0 $\leq x \leq$ 0.2 and temperatures 2 K $\leq T \leq$ 300 K. Data were taken at ambient pressure and finite He-gas pressure $p$ $\leq$ 0.5 GPa. For $x = 0$ and ambient pressure we observe a pronounced valence-change crossover centred around $T'_V$ $\approx$ 160 K with a non-magnetic ground state. This valence-change crossover is characterized by an extraordinarily strong pressure dependence of d$T'_V$ /d$p$ = (80 $\pm 10)$ K/GPa. We observe a shift of $T'_V$ to lower temperatures with increasing Ge-concentration, reaching $T'_V$ $\approx$ 90 K for $x = 0.1$, while still showing a non-magnetic ground state. Remarkably, on further increasing $x$ to 0.2 we find a stable Eu$^{(2+\delta)+}$ valence with long-range antiferromagnetic order below $T_N$ = (47.5 $\pm$ 0.1) K, reflecting a close competition between two energy scales in this system. In fact, by the application of hydrostatic pressure as small as 0.1 GPa, the ground state of this system can be changed from long-range antiferromagnetic order for $p$ $<$ 0.1 GPa to an intermediate-valence state for $p$ $\geq$ 0.1 GPa.

• Investigation of role of antisite disorder in pristine cage compound FeGa$_3$

  C. Kaufmann Ribeiro , L. Mello , V. Martelli , D. Cornejo, M. B. Silva Neto , E. Fogh , H. M. Rønnow, J. Larrea Jiménez

  SciPost Phys. Proc. 11, 023 (2023) · published 5 September 2023 | Toggle abstract · pdf

  The role of controlled Fe antisite disorder in the narrow gap semiconductor FeGa$_3$ has been investigated. Polycrystalline samples were synthesized by the combination of arc-melting furnace and successive annealing processes. Deviations from occupation numbers of Fe and Ga sites expected in the pristine compound were obtained from X-ray data using Rietveld refinement analysis. Besides that, electrical transport and magnetization measurements reveal that hierarchy in Fe and Ga site disorder tunes the ground state of FeGa$_3$ from paramagnetic semiconductor to a magnetic metal. These findings are discussed inside the framework of Anderson localization in the vicinity of metal-semiconductor transitions and spin fluctuations.